Synthesis evidence

Crystal structure and carrier transport properties of a new semiconducting 2D coordination polymer with a 3,5-dimethylpiperidine dithiocarbamate ligand

Okubo T., Anma H., Tanaka N. et al. · Chemical Communications · 2013 · 4316-4318

1 structured synthesis route

Completeness describes how fully the route could be reconstructed from the main article and supporting information.

Partial recipeSource: Both

Route 1: Other

1 · Experimental Section - Synthesis

Metal precursorsCuBr.S(CH3)2; CuII(3,5-Dmpip-dtc)2
Linker precursors3,5-Dmpip-dtc supplied in CuII(3,5-Dmpip-dtc)2 precursor
Solvents10 ml acetonitrile, 10 ml acetone, 20 ml CHCl3; recrystallisation with hexane
Atmospherenot reported
Temperature40
Oxidant / reductantMixed CuI/CuII precursors; no separate oxidant or reductant reported
Work-upStirred 5 min, filtered, then black single crystals obtained in a couple of days by recrystallisation with hexane at 40 deg C.
Activationnot reported
Scalability contextSingle-crystal recrystallisation route; no yield or scale-up data reported.
Show 7 structured reagent records
RoleReagentAmount / concentrationSource
Metal SourceCuBr.S(CH3)20.041 g, 0.2 mmol · in 10 ml acetonitrile, diluted with 10 ml acetone1 · Experimental Section - Synthesis
Metal SourceCuII(3,5-Dmpip-dtc)20.041 g, 0.10 mmol · in 20 ml CHCl31 · Experimental Section - Synthesis
Linker3,5-Dmpip-dtc in CuII(3,5-Dmpip-dtc)2contained in 0.041 g, 0.10 mmol CuII(3,5-Dmpip-dtc)21 · Experimental Section - Synthesis
Solventacetonitrile10 ml1 · Experimental Section - Synthesis
Solventacetone10 ml1 · Experimental Section - Synthesis
SolventCHCl320 ml1 · Experimental Section - Synthesis
Solventhexaneused for recrystallisation1 · Experimental Section - Synthesis