Synthesis evidence

Immobilizing Redox-Active Tricycloquinazoline into a 2D Conductive Metal–Organic Framework for Lithium Storage

Yan J., Cui Y., Xie M. et al. · Angewandte Chemie - International Edition · 2021 · 24467-24472

3 structured synthesis routes

Completeness describes how fully the route could be reconstructed from the main article and supporting information.

Complete recipeSource: Both

Route 1: Solvothermal

SI S4 / rendered p005 · 2.3 Synthesis of Cu-HHTQ · Scheme S2

Metal precursorsCuSO4*5H2O (45 mg, 0.18 mmol)
Linker precursorsHHTQ (50 mg, 0.12 mmol)
Solvents1 mL N,N-dimethylformamide (DMF) plus 2 mL deionised water
AtmosphereSealed 10 mL scintillation vial; no inert gas specified.
Temperature85
Time24
Oxidant / reductantCu(II) salt; O2 shown in Scheme S2 as part of oxidative framework formation.
Work-upCollected by suction filtration using 0.45 um nylon membrane; washed twice with DMF, deionised water, ethanol, and acetone.
ActivationDried in vacuum at 120 C overnight.
Scalability contextSmall-vial batch recipe; no scale-up information reported.
Show 5 structured reagent records
RoleReagentAmount / concentrationSource
LinkerHHTQ50 mg, 0.12 mmolSI S4 / rendered p005 · 2.3 Synthesis of Cu-HHTQ · Scheme S2
SolventN,N-dimethylformamide (DMF)1 mLSI S4 / rendered p005 · 2.3 Synthesis of Cu-HHTQ · Scheme S2
Metal SourceCuSO4*5H2O45 mg, 0.18 mmolSI S4 / rendered p005 · 2.3 Synthesis of Cu-HHTQ · Scheme S2
Solventdeionized water2 mLSI S4 / rendered p005 · 2.3 Synthesis of Cu-HHTQ · Scheme S2
Othernylon membranepore size 0.45 umSI S4 / rendered p005 · 2.3 Synthesis of Cu-HHTQ · Scheme S2
Vague recipeSource: SI

Route 2: Unknown

SI S3 / rendered p004 · 2.2 Synthesis of HHTQ

Vague recipeSource: SI

Route 3: Other

SI S3 / rendered p004 · 2.1 Synthesis of TQ · Scheme S1

Linker precursorsPrecursor structure shown in Scheme S1; exact name and quantities not given in text layer.
AdditivesZnCl2 shown in Scheme S1.
Temperature350
Show 1 structured reagent record
RoleReagentAmount / concentrationSource
AdditiveZnCl2Not specifiedSI S3 / rendered p004 · 2.1 Synthesis of TQ · Scheme S1