Synthesis evidence

Tunable electrical conductivity of a new 3D MOFs: Cu-TATAB

Huang Q.-Q., Lin Y.-J., Zheng R. et al. · Inorganic Chemistry Communications · 2019 · 119-124

2 structured synthesis routes

Completeness describes how fully the route could be reconstructed from the main article and supporting information.

Complete recipeSource: Main

Route 1: Solvothermal

2 · 2.2. Synthesis of Cu-TATAB crystals

Metal precursorsCu(NO3)2.3H2O (0.2 mmol, 25.4 mg)
Linker precursorsH3TATAB (0.1 mmol, 25.7 mg)
SolventsDMF (5 mL), H2O (3 mL), MeOH (2 mL)
AdditivesAcetic acid glacial (350 uL)
AtmosphereNot specified
Temperature125
Time72; cooled to room temperature over 24 h
Work-upGreen crystals collected and washed by DMF four times.
ActivationSoaked in methanol for one week to remove solvent inside the channels.
Scalability context25 mL Teflon-lined reaction vessel; no yield or scale-up data reported.
Show 6 structured reagent records
RoleReagentAmount / concentrationSource
Metal SourceCu(NO3)2.3H2O0.2 mmol, 25.4 mg2 · 2.2. Synthesis of Cu-TATAB crystals
LinkerH3TATAB0.1 mmol, 25.7 mg2 · 2.2. Synthesis of Cu-TATAB crystals
SolventDMF5 mL2 · 2.2. Synthesis of Cu-TATAB crystals
SolventH2O3 mL2 · 2.2. Synthesis of Cu-TATAB crystals
SolventMeOH2 mL2 · 2.2. Synthesis of Cu-TATAB crystals
Acidacetic acid350 uL2 · 2.2. Synthesis of Cu-TATAB crystals
Partial recipeSource: Main

Route 2: Other

4 · Results and discussion · Fig. 4a

Metal precursorsActivated Cu-TATAB
Linker precursorsTCNQ
SolventsMethanol
AtmosphereNot specified
TemperatureNot specified
Time72
Oxidant / reductantTCNQ electron acceptor/dopant
Work-upNot specified in the main text.
ActivationCu-TATAB was activated by methanol soaking before TCNQ treatment.
Scalability contextNo TCNQ concentration, amount, temperature, or post-doping wash/dry details are given in the main text.
Show 3 structured reagent records
RoleReagentAmount / concentrationSource
Otheractivated Cu-TATABNot specified4 · Results and discussion · Fig. 4a
OxidantTCNQmethanol solution; concentration not reported4 · Results and discussion · Fig. 4a
SolventmethanolNot specified4 · Results and discussion · Fig. 4a