Computational Modelling — Unveiling high-mobility hot carriers in a two-dimensional conjugated coordination polymer

Measurement evidence

Computational Modelling

Unveiling high-mobility hot carriers in a two-dimensional conjugated coordination polymer · Fu S., Huang X., Gao G. et al. · Nature Materials · 2025 · 1457-1464

1 measurement group · 5 results

Reported values remain attached to the sample, method, conditions, extraction quality and source location that produced them.

DFT using VASP 5.4.1, PAW, HSE06, Grimme-D2; VASPKIT band paths

Cu3BHT DFT valence-state model series · Model

500 eV plane-wave cutoff; 2 x 3 x 4 Gamma-centred K-point grid for geometry optimization; Cu+/Cu2+ states adjusted via NELECT.

Temperature
0 K computational model / not applicable
Atmosphere
not applicable
Geometry
periodic Cu3BHT model
Context
model Cu3BHT framework
Measurement source
3 · Computational details · Supplementary Fig. 7
PropertyReported valueNormalised valueUncertaintyOrigin and qualitySource
DFT bandgap for Cu2+/Cu+ ratio 0:3~0.4 eVText
Approximate
2 · Synthesis and characterization · Fig. 1h
In-plane electron effective mass0.888 m0Text
Exact Reported
11 · Supplementary Fig. 7 · Supplementary Fig. 7
In-plane hole effective mass0.223 m0Text
Exact Reported
11 · Supplementary Fig. 7 · Supplementary Fig. 7
Reduced effective mass used in main-text mobility calculationm* = 0.187 m0Text
Exact Reported
5 · Crossover from non-equilibrium to quasi-equilibrium regime · Fig. 3
Electron-hole reduced effective mass reported in SI0.178 m0Text
Exact Reported
11 · Supplementary Fig. 7 · Supplementary Fig. 7