Computational Modelling — Decoupling Redox Hopping and Catalysis in Metal-Organic Frameworks -based Electrocatalytic CO2 Reduction

Measurement evidence

Computational Modelling

Decoupling Redox Hopping and Catalysis in Metal-Organic Frameworks -based Electrocatalytic CO2 Reduction · Li X., Surendran Rajasree S., Gude V. et al. · Angewandte Chemie - International Edition · 2023 · e202219046

1 measurement group · 5 results

Reported values remain attached to the sample, method, conditions, extraction quality and source location that produced them.

PM6 semi-empirical optimisation in Gaussian 09; FMO analysis in Multiwfn/VMD

PM6 model of CoPc@NU-1000 · Model

Truncated NU-1000 model with one Zr-oxo SBU, eight TBAPy linkers, and one bidentate-anchored macrocycle

Geometry
molecular cluster model
Context
computational model of guest-loaded MOF
Measurement source
6 · Computational methods · Figures 3, 8, S20-S21
PropertyReported valueNormalised valueUncertaintyOrigin and qualitySource
calculated charge-transfer Delta G for CoPc@NU-1000Marked as a best value within this paper0.014 eVText
Exact Reported
8 · References · Reference note 33
calculated charge-transfer Delta G for TPP(Co)@NU-10000.89 eVText
Exact Reported
8 · References · Reference note 33
centre-to-centre distance from CoPc to adjacent TBAPy13.8 AText
Exact Reported
3 · Results and Discussion · Figure 3
centre-to-centre distance from TPP(Co) to adjacent TBAPy12.4 AText
Exact Reported
3 · Results and Discussion · Figure 3
proposed PhTBAPy-to-PhCoPc tunnelling distanceapproximately 8 AapproximatelyText
Approximate
7 · Results and Discussion · Figure 8