Synthesis evidence

A semiconducting uranium-organic framework based on a tetrathiafulvalene derivative

Zhai F., Li H., Gui D. et al. · Dalton Transactions · 2022

1 structured synthesis route

Completeness describes how fully the route could be reconstructed from the main article and supporting information.

Complete recipeSource: Both

Route 1: Solvothermal

SI p001 · Chemicals and synthesis

Metal precursorsUO2(NO3)2.6H2O, 13 mg (0.03 mmol)
Linker precursorstetrathafulvalene-3,4,5,6-tetrakis(4-benzoic acid) (H4TTFTB), 6.9 mg (0.01 reported without unit)
Solvents1.5 mL water and 1.5 mL N,N-dimethylformamide (DMF)
Additives20 uL concentrated HNO3
AtmosphereSealed 10 mL scintillation vial; gas atmosphere not specified.
Temperature120
Time72
Work-upSonicated for 15 min before heating; dark brown crystals collected and washed with DMF and alcohol three times each.
ActivationProducts dried at 60 deg C.
Scalability contextSmall-vial batch synthesis; no yield or scale-up study reported.
Show 5 structured reagent records
RoleReagentAmount / concentrationSource
Linkertetrathafulvalene-3,4,5,6-tetrakis(4-benzoic acid) (H4TTFTB)6.9 mg (0.01)SI p001 · Chemicals and synthesis
Solventwater1.5 mLSI p001 · Chemicals and synthesis
SolventN,N-dimethylformamide (DMF)1.5 mLSI p001 · Chemicals and synthesis
Metal SourceUO2(NO3)2.6H2O13 mg (0.03 mmol)SI p001 · Chemicals and synthesis
Acidconcentrated HNO320 uL · concentratedSI p001 · Chemicals and synthesis