Spectroscopy — Controlling the Spatiotemporal Self-Organization of Stimuli-Responsive Nanocrystals under Out-of-Equilibrium Conditions

Measurement evidence

Spectroscopy

Controlling the Spatiotemporal Self-Organization of Stimuli-Responsive Nanocrystals under Out-of-Equilibrium Conditions · Damacet P., Shehayeb E.O., Mirica K.A. · Journal of the American Chemical Society · 2025 · 1584-1594

2 measurement groups · 7 results

Reported values remain attached to the sample, method, conditions, extraction quality and source location that produced them.

DRIFTS and ex situ XPS after H2S exposure

2D RD Ni3(HITP)2 interface particles · Powder

DRIFTS after exposure to 0.1% H2S in N2 for 30 min; XPS after 1% H2S in N2 for 2 h.

Atmosphere
H2S in N2
Context
pristine 2D RD interface particles before/after analyte exposure
Measurement source
1591 · Figure caption · Figure 6
PropertyReported valueNormalised valueUncertaintyOrigin and qualitySource
DRIFTS C-N stretching shift after H2S exposure, peak 11036 to 1070 cm-1Text
Rounded Reported
1590 · 3.5 Chemiresistive Detection · Figure 6a,b
increase in Ni-N-C to Ni-N=C peak area ratio after gas sensing5-fold increaseText
Rounded Reported
1591 · 3.5 Chemiresistive Detection · Figure 6d
EDX sulfur uptake after 20 ppm H2S, interface-particle electrodeMarked as a best value within this paper3.2 +/- 0.49%+/- 0.49%Text
Rounded Reported
1590 · 3.5 Chemiresistive Detection · Figures S98-S105
EDX sulfur uptake after 20 ppm H2S, Zone 3-particle electrode0.45% +/- 0.11%+/- 0.11%Text
Rounded Reported
1590 · 3.5 Chemiresistive Detection · Figures S98-S105
new XPS S 2p peak assigned to H2S-Ni species163.7 eVText
Rounded Reported
1591 · 3.5 Chemiresistive Detection · Figure 6d

X-ray photoelectron spectroscopy (XPS)

2D RD Ni3(HITP)2 interface particles · Powder

Kratos Analytical AXIS Supra, ultrahigh vacuum, monochromatic Al Kalpha, 200 um beam diameter; survey and high-resolution spectra.

Atmosphere
ultrahigh vacuum
Context
pristine 2D RD-derived framework particles
Measurement source
65 · S10.5 Chemical stability · Figure S80; Table S2
PropertyReported valueNormalised valueUncertaintyOrigin and qualitySource
XPS nickel mass fraction range across 2D zones1.7 to 2.3 mass %Visual Estimate
Range
65 · S10.5 Chemical stability of Ni3(HITP)2 crystals · Table S2
XPS nitrogen atomic fraction range across 2D zones4.2 to 6.4 atomic %Visual Estimate
Range
65 · S10.5 Chemical stability of Ni3(HITP)2 crystals · Table S2