Diffraction Structure — Electrically Conductive π-Intercalated Graphitic Metal-Organic Framework Containing Alternate π-Donor/Acceptor Stacks

Measurement evidence

Diffraction Structure

Electrically Conductive π-Intercalated Graphitic Metal-Organic Framework Containing Alternate π-Donor/Acceptor Stacks · Yadav A., Zhang S., Benavides P.A. et al. · Angewandte Chemie - International Edition · 2023 · e202303819

2 measurement groups · 12 results

Reported values remain attached to the sample, method, conditions, extraction quality and source location that produced them.

PXRD with Rietveld refinement against DFT-optimised model

iGMOF1 black powder · Powder

Cu Kalpha PXRD; Rietveld refinement in Rigaku SmartLab Studio; structural units treated as rigid bodies.

Context
Target framework structure and phase-purity assignment.
Measurement source
S2 · Rietveld Refinement · Figure S2
PropertyReported valueNormalised valueUncertaintyOrigin and qualitySource
HCTP centroid offset from neighbouring HATP ligandscentroid-centroid displacement approx. 0.8 A0.8 angstromapprox.Text
Approximate
4 · Results and Discussion · Figure 2c,d
Calculated HATP/HCTP interplanar distance in iGMOF1dHATP/HCTP approx. 3.3 A3.3 angstromapprox.Text
Approximate
4 · Results and Discussion · Figure 2c,d
iGMOF1 Rietveld RpRp = 5.60 %0.056 fractionFigure Axis
Exact Reported
S5 · Figure S2 · Figure S2
iGMOF1 Rietveld RwpRwp = 7.52 %0.0752 fractionFigure Axis
Exact Reported
S5 · Figure S2 · Figure S2
Rietveld-refined space grouporthorhombic C2mmText
Qualitative
3 · Results and Discussion · Figure S2
Temperature-dependent PXRD stability of iGMOF1crystalline structure remained intact at least up to 100 deg C373.15 Kat leastText
Rounded Reported
6 · Results and Discussion · Figure S13
iGMOF1 Rietveld unit-cell aa = 21.82306 A21.82306 angstromFigure Axis
Exact Reported
S5 · Figure S2 · Figure S2
iGMOF1 Rietveld unit-cell bb = 37.48085 A37.48085 angstromFigure Axis
Exact Reported
S5 · Figure S2 · Figure S2
iGMOF1 Rietveld unit-cell cc = 6.61077 A6.61077 angstromFigure Axis
Exact Reported
S5 · Figure S2 · Figure S2

Single-crystal X-ray diffraction

Supramolecular [HATP/HCTP]n array powder/crystals · Powder

SCXRD of supramolecular [HATP/HCTP]n array; disordered solvent omitted by PLATON/SQUEEZE.

Temperature
100
Context
Precursor/model array used to infer HATP/HCTP orientation in iGMOF1.
Measurement source
S2 · X-Ray Crystallography · Table S1
PropertyReported valueNormalised valueUncertaintyOrigin and qualitySource
HATP/HCTP interplanar distance in supramolecular arraydHATP/HCTP approx. 3.3 A3.3 angstromapprox.Text
Approximate
3 · Results and Discussion · Figure 2a
Supramolecular array formula weight696.73696.73 g mol-1SI Table
Exact Reported
S11 · Table S1 · Table S1
Supramolecular array crystal system and space groupMonoclinic, CcSI Table
Exact Reported
S11 · Table S1 · Table S1