Diffraction Structure — Constructing a Redox-Active Cu(I)-Pyridyltriazine Framework for Catalytic Photoreduction of Nitrobenzenes and Carboxylic Cyclization of Alkynol with CO2

Measurement evidence

Diffraction Structure

Constructing a Redox-Active Cu(I)-Pyridyltriazine Framework for Catalytic Photoreduction of Nitrobenzenes and Carboxylic Cyclization of Alkynol with CO2 · Zhang T., Si C., Guo K. et al. · Inorganic Chemistry · 2022 · 20657-20665

1 measurement group · 12 results

Reported values remain attached to the sample, method, conditions, extraction quality and source location that produced them.

Single-crystal X-ray diffraction, Bruker APEX-II CCD, Mo Kalpha radiation

As-synthesised Cu(I)-TPT orange rhombus single crystals · Single Crystal

Single crystal sealed in a glass tube; data collected at 150 K; solved with Olex2 and refined by Gauss-Newton minimisation.

Temperature
150
Geometry
single crystal
Context
pristine framework
Measurement source
S2 · 1.2.1 Crystallography · Tables S1-S2
PropertyReported valueNormalised valueUncertaintyOrigin and qualitySource
Cu(I)-CN bond-length range1.868 to 1.885 AText
Range
p002 / 20658 · Synthesis and Crystal Structure · Figure 2 and Table S2
Cu(I)-N(TPT) bond-length range2.056 to 2.078 AText
Range
p003 / 20659 · Synthesis and Crystal Structure · Figure 2 and Table S2
Empirical formulaC25H18Cu3N11SI Table
Exact Reported
S2 · 1.2.1 Crystallography · Table S1
Typical C-H...(CN) hydrogen-bond distanceabout 2.8080 A2.808 AText
Approximate
p003 / 20659 · Synthesis and Crystal Structure · Figure S1b
Pi-pi stacking interaction distanceabout 3.3-3.4 AText
Approximate
p003 / 20659 · Synthesis and Crystal Structure · Figure 2c-e
Final R1 index for I >= 2sigma(I)R1 = 0.03330.0333SI Table
Exact Reported
S3 · Table S1 · Table S1
Space groupC2/cSI Table
Exact Reported
S3 · Table S1 · Table S1
Unit-cell a11.8159(5) A11.8159 A(5)SI Table
Exact Reported
S3 · Table S1 · Table S1
Unit-cell b18.4055(7) A18.4055 A(7)SI Table
Exact Reported
S3 · Table S1 · Table S1
Unit-cell beta angle115.065(1) degree115.065 degree(1)SI Table
Exact Reported
S3 · Table S1 · Table S1
Unit-cell c13.4717(6) A13.4717 A(6)SI Table
Exact Reported
S3 · Table S1 · Table S1
Unit-cell volume2653.9(2) A32653.9 A3(2)SI Table
Exact Reported
S3 · Table S1 · Table S1