Diffraction Structure — A new semiconducting coordination polymer consisting of copper(I)-iodide and 3-pyridinecarboxaldehyde

Measurement evidence

Diffraction Structure

A new semiconducting coordination polymer consisting of copper(I)-iodide and 3-pyridinecarboxaldehyde · Himoto K., Horii T., Syoji T. et al. · Inorganic Chemistry Communications · 2018 · 34-37

2 measurement groups · 34 results

Reported values remain attached to the sample, method, conditions, extraction quality and source location that produced them.

Single-crystal X-ray diffraction

Yellow needle-shaped single crystals of 1 · Single Crystal

Rigaku R-AXIS RAPID imaging plate detector; graphite-monochromated Mo-Kalpha radiation; 44 oscillation images; numerical absorption correction; solved by direct methods and refined with SHELXL97.

Temperature
100
Geometry
Single crystal; CIF crystal size 0.300 x 0.200 x 0.200 mm.
Context
pristine_framework
Measurement source
1.3. X-ray structure determination · Table S5; CIF
PropertyReported valueNormalised valueUncertaintyOrigin and qualitySource
Bond valence sum for Cu1.12Text
Exact Reported
main p.1 / article p.34 · Structure discussion
Unit cell aa = 4.1245(4) A(4)Table
Exact Reported
Crystal data · CIF _cell_length_a
Unit cell alphaalpha = 96.719(3) deg(3)Table
Exact Reported
Crystal data · CIF _cell_angle_alpha
Unit cell bb = 7.6624(6) A(6)Table
Exact Reported
Crystal data · CIF _cell_length_b
Unit cell betabeta = 92.504(3) deg(3)Table
Exact Reported
Crystal data · CIF _cell_angle_beta
Unit cell cc = 12.3687(9) A(9)Table
Exact Reported
Crystal data · CIF _cell_length_c
Unit cell gammagamma = 100.643(2) deg(2)Table
Exact Reported
Crystal data · CIF _cell_angle_gamma
Unit cell volumeV = 380.67(5) A3(5)Table
Exact Reported
Crystal data · CIF _cell_volume
Crystal systemtriclinicTable
Exact Reported
SI p.S10 · Table S5 · Table S5
Nearest-neighbour Cu-Cu separation 12.7490(4) A(4)Text
Exact Reported
main p.1 / article p.34 · Structure discussion · Fig. 1
Nearest-neighbour Cu-Cu separation 22.7791(4) A(4)Text
Exact Reported
main p.1 / article p.34 · Structure discussion · Fig. 1
CIF Cu-I bond length 1I1-Cu1 = 2.6078(4) A(4)Table
Exact Reported
Molecular geometry · CIF _geom_bond_distance
CIF Cu-I bond length 2I1-Cu1 = 2.6283(4) A(4)Table
Exact Reported
Molecular geometry · CIF _geom_bond_distance
CIF Cu-I bond length 3I1-Cu1 = 2.6931(4) A(4)Table
Exact Reported
Molecular geometry · CIF _geom_bond_distance
Average Cu-I bond length2.6317(4) A(4)Text
Exact Reported
main p.1 / article p.34 · Structure discussion · Fig. 1
Cu-N bond lengthCu1-N1 = 2.055(2) A(2)Table
Exact Reported
Molecular geometry · CIF _geom_bond_distance
Calculated densityDcalc = 2.596 g/cm3Table
Exact Reported
SI p.S10 · Table S5 · Table S5
Maximum residual electron-density peak0.71 e/A3Table
Exact Reported
SI p.S11 · Table S5 · Table S5
Minimum residual electron-density peak-1.92 e/A3Table
Exact Reported
SI p.S11 · Table S5 · Table S5
Framework dimensionalityone-dimensional infinite ladder chainText
Qualitative
main p.1 / article p.34 · Structure discussion · Fig. 1
F000276.00Table
Exact Reported
SI p.S11 · Table S5 · Table S5
Empirical formulaC6H5CuINOTable
Exact Reported
SI p.S10 · Table S5 · Table S5
Formula weight297.56Table
Exact Reported
SI p.S10 · Table S5 · Table S5
Goodness of fit indicator1.129Table
Exact Reported
SI p.S11 · Table S5 · Table S5
Linear absorption coefficient for Mo-Kalpha68.500 cm-1Table
Exact Reported
SI p.S11 · Table S5 · Table S5
3-Py-CHO plane separation3.476 AText
Exact Reported
main p.1 / article p.34 · Structure discussion · Fig. S2
R factor for observed reflectionsR (I > 2.00 sigma(I)) = 0.0246Table
Exact Reported
SI p.S11 · Table S5 · Table S5
Number of refined variables91Table
Exact Reported
SI p.S11 · Table S5 · Table S5
RintRint = 0.0348Text
Exact Reported
1.3. X-ray structure determination
Space groupP-1 (#2)Table
Exact Reported
SI p.S10 · Table S5 · Table S5
Unique reflections1723 were uniqueText
Exact Reported
1.3. X-ray structure determination
Weighted R factor for all reflectionswR = 0.0636Table
Exact Reported
SI p.S11 · Table S5 · Table S5
Z valueZ = 2Table
Exact Reported
Crystal data · CIF _cell_formula_units_Z

Powder X-ray diffraction comparison with calculated pattern

Powdered sample of [CuI(3-Py-CHO)]n · Powder

Experimental XRPD pattern for 1 compared with calculated pattern from single-crystal data.

Geometry
Powder sample
Context
pristine_framework
Measurement source
SI p.S4 · Supporting figures · Figure S3
PropertyReported valueNormalised valueUncertaintyOrigin and qualitySource
XRPD pattern comparisonExperimental XRPD pattern of 1 compared with calculated pattern from single-crystal data.Caption
Qualitative
SI p.S4 · Supporting figures · Figure S3