Computational Modelling — Phosphonate Metal–Organic Frameworks: A Novel Family of Semiconductors

Measurement evidence

Computational Modelling

Phosphonate Metal–Organic Frameworks: A Novel Family of Semiconductors · Siemensmeyer K., Peeples C.A., Tholen P. et al. · Advanced Materials · 2020 · 2000474

1 measurement group · 12 results

Reported values remain attached to the sample, method, conditions, extraction quality and source location that produced them.

ADF2018 BAND periodic DFT; PBE-D3-BJ geometry optimisation; HSE06 single-point calculations; STO basis sets.

TUB75 1x3x1 periodic DFT supercell · Model

1x3x1 periodic supercell; TZP STO basis for Cu, DZP STO basis for main group atoms; Gamma-point sampling; spin-polarised unrestricted Kohn-Sham DFT.

Geometry
periodic 1x3x1 supercell
Context
model of pristine TUB75
Measurement source
2 · Density functional theory calculations
PropertyReported valueNormalised valueUncertaintyOrigin and qualitySource
average partial charge C Hirshfeld-0.022-0.022 elementary chargeSI Table
Exact Reported
15 · Table S2 · Table S2
average partial charge Cu CM50.8670.867 elementary chargeSI Table
Exact Reported
15 · Table S2 · Table S2
average partial charge Cu Hirshfeld0.5360.536 elementary chargeSI Table
Exact Reported
15 · Table S2 · Table S2
average partial charge Cu Mulliken0.9210.921 elementary chargeSI Table
Exact Reported
15 · Table S2 · Table S2
average partial charge Cu Voroni0.5610.561 elementary chargeSI Table
Exact Reported
15 · Table S2 · Table S2
average partial charge H Hirshfeld0.0390.039 elementary chargeSI Table
Exact Reported
15 · Table S2 · Table S2
average partial charge N Hirshfeld-0.090-0.09 elementary chargeSI Table
Exact Reported
15 · Table S2 · Table S2
average partial charge O Hirshfeld-0.331-0.331 elementary chargeSI Table
Exact Reported
15 · Table S2 · Table S2
average partial charge P Hirshfeld0.4560.456 elementary chargeSI Table
Exact Reported
15 · Table S2 · Table S2
DFT HOMO-LUMO gapEg = 1.77 eV1.77 eVText
Exact Reported
3 · main text
DFT exchange energy AFM minus FMMarked as a best value within this paperEex = EAFM - EFM = -37.3 meV-37.3 meVText
Exact Reported
4 · main text
spin density isosurface level0.005 electrons per Angstrom30.005 electrons Angstrom-3Caption
Exact Reported
6 · caption · Figure 6