Computational Modelling — Electron-Conductive Metal-Organic Framework, Fe(dhbq)(dhbq = 2,5-Dihydroxy-1,4-benzoquinone): Coexistence of Microporosity and Solid-State Redox Activity

Measurement evidence

Computational Modelling

Electron-Conductive Metal-Organic Framework, Fe(dhbq)(dhbq = 2,5-Dihydroxy-1,4-benzoquinone): Coexistence of Microporosity and Solid-State Redox Activity · Kon K., Uchida K., Fuku K. et al. · ACS Applied Materials and Interfaces · 2021 · 38188-38193

1 measurement group · 3 results

Reported values remain attached to the sample, method, conditions, extraction quality and source location that produced them.

DFT structural optimisation and calculated UV-Vis-NIR/orbitals

Fe dimer computational model · Model

Dimer model {Fe(Hdhbq)2}2 and Fe2(dhbq)(Hdhbq)2(H2O)4 frontier orbitals; code/functional not specified in extracted text

Measurement source
12 · Optimized structure · Figures S9, S12, S13
PropertyReported valueNormalised valueUncertaintyOrigin and qualitySource
calculated main absorption assignmentmain absorption band attributed mainly to HOMO-to-LUMO transitionCaption
Qualitative
15 · Calculated UV-Vis-NIR spectra · Figure S12
DFT-optimised axial coordinationoxygen atom of dhbq coordinates to one side of axial siteText
Qualitative
3 · Results and Discussion · Figure S9
EXAFS RDF fit R-factorR-factor was 0.0163Text
Exact Reported
13 · RDF fitting · Figure S10